W0249

Crystallographic Studies of the Human Prion Protein. Karen J. Knaus1,2, Rune Hartmann1, Lizamma Antony1, David Vanik3, Manuel Morillas3, Wieslaw Swietnicki3, Witold K. Surewicz3,5,6 and Vivien C. Yee1,2,4, 1Dept. of Molecular Cardiology and Center for Structural Biology, Lerner Research Institute, Cleveland Clinic Foundation, 2Dept. of Chemistry, Cleveland State Univ., Depts. of 3Pathology, 4Pharmacology, 5Chemistry and 6Physiology and Biophysics, Case Western Reserve Univ.

Prions are novel infectious particles that are believed to be composed entirely of proteins. They have been found to play an important role in the pathogenesis of neurodegenerative diseases that can be infectious, inherited, and sporadic. The key event in disease transmission is believed to be the structural conversion of PrPC (predominantly α-helical, monomeric form) to PrPSc (predominantly β-sheet enriched, oligomeric form of the protein). During the conversion of PrPC to PrPSc, it is believed that the protein obtains a marked increase in β-sheet secondary structure. The predominantly β-sheet PrPSc isoform can then further oligomerize and eventually deposit itself as fibrils, β-amyloid plaques, or other insoluble aggregates in the brains of diseased patients. Many recent investigations of PrP have been targeted at studying the differences between the two isoforms and their respective roles in the PrPC to PrPSc conversion. Thus structural studies of the prion protein (PrP) seem to be a logical starting point for understanding prion disease mechanism. Previously determined high resolution NMR structures of bacterially expressed PrP from mouse, hamster, cow and human have been useful in determining a monomeric predominantly α-helical state of the protein. Our crystallographic studies of recombinant human prion proteins, focusing on wild-type and pathogenic mutants, reveals additional structural features which may be important in understanding the PrPC to PrPSc conversion and/or aggregation properties of the protein.